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Triple Spin Interaction and Entanglement

Willi-Hans Steeb

International School for Scientific Computing, University of Johannesburg, Auckland Park 2006, South Africa

Reprint requests to W.-H. S.; E-mail:steebwilli@gmail.com

Z. Naturforsch.68a,172 – 177 (2013) / DOI: 10.5560/ZNA.2012-0087 Received September 20, 2012 / published online February 15, 2013

We study a Hamilton operator ˆH for spin-1/2 with triple spin interactions. The eigenvalues and eigenvectors are determined and the unitary matrices exp(−i ˆHt/¯h)are found. Entanglement of the eigenvectors is investigated. A Hamilton operator ˆK for spin-1 and triple spin interaction is also discussed.

Key words:Spin Interactions; Hamilton Operators; Entanglement.

1. Introduction

In quantum theory Hamilton operators with spin- interactions have a long history [1–5]. Triple spin in- teraction have been studied by several authors [6–19].

Igl´oi [6] investigated an Ising model with three-spin interaction by finite-size scaling and applying free boundary conditions. Vanderzande and Igl´oi [7] stud- ied the critical behaviour and logarithmic corrections of a quantum model with three-spin interaction. Al- caraz and Barber [8] and Wittlich [9] studied a one- dimensional Ising quantum chain with 3N sites with staggered three-spin coupling and periodic boundary conditions. Somma et al. [10] studied the unitary oper- atorU(t) =exp(iωtσ1⊗σ3⊗σ2). Hereσ123are the Pauli spin matrices

σ1= 0 1

1 0

, σ2=

0 −i

i 0

, σ3=

1 0 0 −1

. Pachos and Plenio [11] studied three-spin interac- tions in optical lattices. Three qubit Hamilton oper- ators and Riemannian geometry has been discussed by Brandt [12]. Using the mean field method Jiang and Kong [13] studied a spin-1 quantum Ising model with three-spin interaction. Wang et al. [14] investi- gated the bifurcation in ground-state fidelity for a one- dimensional spin model with competing two-spin and three-spin interactions. Lanyon et al. [15] considered among others the triple-spin operatorσ3⊗σ1⊗σ1for universal digital quantum simulation with trapped ions.

Topilko et al. [16] considered magnetocaloric effects in

spin-1/2 XX chains with three-spin interactions. Zhang et al. [17] investigated the geometric phase of a qubit symmetrically coupled to a XY-spin chain with three spin interaction in a transverse magnetic field. The Greenberger–Horne–Zeilinger (GHZ) state and triple- spin operatorsσ1⊗σ2⊗σ22⊗σ1⊗σ22⊗σ2⊗ σ11⊗σ1⊗σ1have been discussed by Aravind [18]

in connection with Bell’s theorem without inequalities.

A nonlinear eigenvalue problem with triple-spin inter- action has been solved by Steeb and Hardy [19]. Here we consider triple-spin interaction and entanglement for spin-1/2 systems. Spin-1 systems will also be dis- cussed.

We consider the Hamilton operator with triple-spin interaction of spin-1/2,

Hˆ =¯ 11I2⊗I2+I2⊗σ2⊗I2+I2⊗I2⊗σ3) +¯ 21⊗σ2⊗I21I2⊗σ3+I2⊗σ2⊗σ3) +¯ 31⊗σ2⊗σ3),

whereσ1, σ23 are the Pauli spin matrices, and I2

is the 2×2 unit matrix. Thus the Hamilton operator Hˆ acts in the Hilbert spaceC8. The Pauli matrices are hermitian and unitary withσ122232=I2. The eigenvalues are+1 and−1 with the corresponding nor- malized eigenvectors

u1= 1

√ 2

1 1

, u−1= 1

√ 2

1

−1

, v1= 1

√2 1

i

, v−1= 1

√2 1

−i

,

© 2013 Verlag der Zeitschrift f¨ur Naturforschung, T¨ubingen·http://znaturforsch.com

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w1= 1

0

, w−1= 0

1

.

We calculate the unitary matrixU(t) =exp(−i ˆHt/h)¯ to solve the Schr¨odinger and Heisenberg equation of motion. These unitary operators are applied to en- tangled and unentangled states. Entangled and un- entangled states can be found depending on the pa- rameters ¯1, ¯2, ¯3. As entanglement measure for the Hamilton operator ˆH, we consider the three- tangle.

2. A Theorem

For the calculation of the eigenvalues and eigenvec- tors of the Hamilton operator ˆH, we utilize the follow- ing theorem [20,21]. LetA1,A2,A3ben×nmatrices over CandInbe then×nunit matrix. Consider the matrix

M=c1(A1In⊗In+InA2In+InInA3) +c2(A1A2⊗In+A1InA3+In⊗A2A3) +c3(A1A2⊗A3),

wherec1, c2,c3are constants. Since the terms in M commutate pairwise, we can write exp(M)as

eM=ec1A1⊗In⊗Inec1In⊗A2⊗Inec1In⊗In⊗A3ec2A1⊗A2⊗In

·ec2A1⊗In⊗A3ec2In⊗A2⊗A3ec3(A1⊗A2⊗A3).

If|ui,|vi,|wiare eigenvectors ofA1,A2,A3, respec- tively, with eigenvaluesλ,µ,ν, we find the eigenvec- tor|ui ⊗ |vi ⊗ |wiofMwith the eigenvalue

c1(λ+µ+ν) +c2(λ µ+λ ν+µ ν) +c3(λ µ ν).

Then|ui ⊗ |vi ⊗ |wiis also an eigenvector of eMwith the corresponding eigenvalues

c1(λ+µ+ν) +c2(λ µ+λ ν+µ ν) +c3(λ µ ν).

If the matricesA1,A2,A3have the additional properties that A21=A22=A23=In(spin-12 case withn=2), we obtain

ec3A1⊗A2⊗A3= (InIn⊗In)cosh(c3) + (A1A2A3)cosh(c3).

If the matricesA1,A2,A3have the additional properties thatA3j=Aj with j=1,2,3 (spin-1 case withn=3), we obtain

ec3A1⊗A2⊗A3=InInIn+ (A1⊗A2⊗A3)sinh(c3) + (A21A22A23)(cosh(c3)−1). 3. Spin-1/2 Case

The eight normalized eigenvectors of ˆHcan be con- structed from the normalized eigenvectors of σ12, σ3and the Kronecker products

e111=u1⊗v1w1, e11−1=u1v1⊗w−1, e1−11=u1v−1w1, e1−1−1=u1⊗v2w2, e−111=u−1⊗v1w1, e−11−1=u−1v1w−1, e−1−11=u−1v−1⊗w1, e−1−1−1=u−1v−1w−1

with the corresponding eight eigenvalues E111=h(3ω¯ 1+3ω23), E11−1=h(ω¯ 1−ω2−ω3), E1−11=h(ω¯ 1−ω2−ω3), E1−1−1=h(−ω¯ 1−ω23), E−111=h(ω¯ 1−ω2−ω3), E−11−1=h(−ω¯ 1−ω23), E−1−11=h(−ω¯ 1−ω23), E−1−1−1=h(−3ω¯ 1+3ω2−ω3),

whereE11−1=E1−11=E−111andE1−1−1=E−11−1= E−1−11. The eigenvaluesE111andE−1−1−1are not de- generate. Note that the eight normalized eigenvectors are pairwise orthogonal. Thus we have (spectral de- composition)

Hˆ=

j,k,`∈{1,−1}

Ejk`ejk`ejk`.

Now the unitary matrixU(t) = e−itH/¯ˆ h can be con- structed from the normalized eigenvectors and eigen- values of ˆHvia

e−itH/¯ˆ h=

j,k,`∈{1,−1}

e−iEjk`t/¯hejk`ejk`.

We find

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U(t) =

u11(t) 0 u13(t) 0 u15(t) 0 u17(t) 0 0 u22(t) 0 u24(t) 0 u26(t) 0 u28(t) u31(t) 0 u33(t) 0 u35(t) 0 u37(t) 0

0 u42(t) 0 u44(t) 0 u46(t) 0 u48(t) u51(t) 0 u53(t) 0 u55(t) 0 u57(t) 0

0 u62(t) 0 u64(t) 0 u66(t) 0 u66(t) u71(t) 0 u73(t) 0 u75(t) 0 u77(t) 0

0 u82(t) 0 u84(t) 0 u86(t) 0 u88(t)

with

u11(t) =u33(t) =u55(t) =u77(t)

= e−iE1t/¯h/4+e−iE2t/¯h/2+e−iE4t/¯h/4, u13(t) =−u31(t) =−i e−iE1t/¯h/4+i e−iE4t/¯h/4, u15(t) =u51(t) =e−iE1t/¯h/4−e−iE4t/¯h/4, u17(t) =−u71(t)

=−i e−iE1t/¯h/4−i e−iE4t/¯h/4+i e−iE2t/¯h/2, u22(t) =u44(t) =u66(t) =u88(t)

=e−iE2t/¯h/4+e−iE4t/¯h/2+e−iE8t/¯h/4, u24(t) =−u42(t) =−i e−iE2t/¯h/4+i e−iE8t/¯h/4, u26(t) =u62=e−iE2t/¯h/4−e−iE8t/¯h/4,

u28(t) =−u82

=−i e−iE2t/¯h/4+i e−iE4t/¯h/2−i e−iE8t/¯h/4, u35(t) =−u53

=i e−iE1t/¯h4−i e−iE2t/¯h/2+i e−iE4t/¯h/4, u37(t) =u73=e−iE1t/¯h/4−e−iE4t/¯h/4,

u46(t) =−u64

=i e−iE2t/¯h/4−i e−iE4t/¯h/2+i e−iE8t/¯h, u48(t) =u84=e−iE2t/¯h/4−i e−iE8t/¯h/4, u57(t) =−u75=−i e−iE1t/¯h/4+i e−iE4t/¯h/4, u68(t) =−u86=−i e−iE2t/¯h/4+i e−iE8t/¯h/4

with 1↔111, 2↔11−1, 3↔1−11, 4↔1−1−1, 5↔ −111, 6↔ −11−1, 7↔ −1−11, 8↔ −1−1− 1.

4. Entanglement

Entangled quantum states are an important compo- nent of quantum computing techniques such as quan- tum error-correction, dense coding, and quantum tele- portation [21–27]. Entanglement is the characteristic

trait of quantum mechanics which enforces its entire departure from classical lines of thought. We consider entanglement of pure states. Entanglement of Hamil- ton operators with triple-spin interaction has not been considered so far.

The eigenvectors given above are product states and hence not entangled. However, some of the eigenvalues are degenerate(E2=E3=E5andE4=E6=E7)and thus we can form linear combinations of these eigen- vectors which are again eigenvectors and can be entan- gled.

An N-tangle can be defined for the finite dimen- sional Hilbert spaceH=C2

N, withN=3 orN even.

Two-level and higher-level quantum systems and their physical realization have been studied by many au- thors. We consider the finite-dimensional Hilbert space H=C2

N and the normalized states

|ψi=

1 j1,j2,...,

jN=0

cj1,j2,...,jN|j1i ⊗ |j2i ⊗ · · · ⊗ |jNi

in this Hilbert space. Here|0i,|1idenotes the standard basis. Letεjk(j,k=0,1)be defined byε0011=0, ε01=1,ε10=−1. LetN be even orN=3. Then an N-tangle can be introduced by [27]

τ1...N=2

1

α1,...,αN=0 ...

δ1,...,δN=0

cα1...αNcβ1...βNcγ1...γncδ1...δN

·εα1β1εα2β2· · ·εαN−1βN−1εγ1δ1εγ2δ2

· · ·εγN−1δN−1εαNγNεβNδN .

This includes the definition for the 3-tangle withN= 3. A computer algebra program to find theN-tangle is given by Steeb and Hardy [28].

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ConsiderN=3 and the GHZ-state and theW-state

|GHZi= 1

√ 2

 1 0 0 0 0 0 0 1

, |Wi= 1

√ 3

 0 1 1 0 1 0 0 0

 .

Then we find for the GHZ-state thatτ=1 andτ=0 for theW-state. Note that the|Wistate is not separable.

Consider the triple-spin interaction Hamilton opera- tor

HˆT

¯

1⊗σ2⊗σ3.

The eigenvalues are +1 (fourfold) and−1 (fourfold).

A set of normalized eigenvectors are the separable states (and thus not entangled) given above. Owing to the degeneracy of the eigenvalue+1 (and analogously for the eigenvalue−1), we can form linear combina- tions of these separable eigenstates that are fully entan- gled. From the four separable eigenstates with eigen- value+1

1 1

⊗ 1

1

⊗ 1

1 1 1

⊗ 1

1

⊗ 1

1 1

1

⊗ 1

1

⊗ 1

1 1 1

⊗ 1

1

⊗ 1

1

,

we find by linear combinations the fully entangled eigenstates (using the three tangle described above) with eigenvalue+1

1 2

 1 1 0 0 0 0 i

−i

 , 1

2

 0 1 i 0 1 0 0

−i

 , 1

2

 0 0 i

−i 1 1 0 0

 , 1

2

 0 1 i 0 1 0 0 i

 .

The four vectors are also linearly independent. Anal- ogously we can make this construction for the eigen- value −1 to find fully entangled states, i. e. the three tangle isτ= +1.

5. Spin-1 Case

Consider the Hamilton operator with triple-spin in- teraction with spin-1 system with the Hamilton opera- tor

Kˆ=¯ 1(s1I3I3+I3⊗s2⊗I3+I3I3⊗s3) +¯ 2(s1s2I3+s1⊗I3s3+I3⊗s2⊗s3) +¯ 3(s1s2s3),

wheres1,s2,s3are the trace-less and hermitian 3×3 matrices

s1= 1

√2

0 1 0

1 0 1

0 1 0

, s2= 1

√2

0 −i 0

i 0 −i

0 i 0

,

s3=

1 0 0

0 0 0

0 0 −1

,

andI3is the 3×3 identity matrix. The Hamilton op- erator ˆK acts in the Hilbert spaceC27. Here one can investigate whether the state inC27 can be written as a product state of two vectors inC9 andC3,C3 and C9, orC3,C3andC3. Note thats3j=sjfor j=1,2,3 and thuss4j=s2j for j=1,2,3. The eigenvalues of the matricess1,s2,s3are given by+1, 0,−1. The normal- ized eigenvectors fors1are

u1=1 2

√1 2 1

, u0= 1

√ 2

 1 0

−1

,

u−1=1 2

 1

−√ 2 1

.

The normalized eigenvectors fors2are

v1=1 2

√1 2i

−1

, v0= 1

√ 2

 1 0 1

,

v−1=1 2

 1

−√ 2i

−1

.

The normalized eigenvectors fors3is the standard ba- sis denoted byw1,w0,w−1. Thus the 27 normalized eigenvectors (separable states) are given by

ejk`=uj⊗vk⊗w`, j,k, `=1,0,−1

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with the 27 eigenvalues

Ejk`=¯ 1(j+k+`) +¯ 2(jk+j`+k`) +¯ 3(jk`).

Now for the unitary matrixV(t) =e−itK/¯ˆ h, we find V(t) =

j,k,`∈{1,0,−1}

e−iEjk`t/¯hejk`ejk`. Note that forz∈C, we have

ezs1⊗I3⊗I3=I3I3I3+ (s1I3⊗I3)sinh(z) + (s21⊗I3I3)(cosh(z)−1), ezs1⊗s2⊗I3=I3I3⊗I3+ (s1s2I3)sinh(z)

+ (s21⊗s22⊗I3)(cosh(z)−1), ezs1⊗s2⊗s3=I3I3⊗I3+ (s1s2⊗s3)sinh(z)

+ (s21⊗s22⊗s23)(cosh(z)−1).

Withz=−iωt, we arrive at

e−iωts1⊗s2⊗s3 =I3I3I3−i(s1s2s3)sin(ωt) + (s21s22⊗s23)(cos(ωt)−1).

For ω1=0, ω2=0, the eigenvalues are highly de- generate, and we can form eigenvectors which are entangled.

6. Conclusion

We have studied spin Hamilton operators with triple-spin interaction. If the eigenvalues are degener- ate then by linear combinations, we can construct en- tangled states from unentangled states.

Acknowledgement

The author is supported by the National Research Foundation (NRF), South Africa. This work is based upon research supported by the National Research Foundation. Any opinion, findings and conclusions or recommendations expressed in this material are those of the author(s) and therefore the NRF do not accept any liability in regard thereto.

[1] W. Heisenberg, Z. Physik46, 619 (1928).

[2] H. Bethe, Z. Physik71, 205 (1931).

[3] L. Onsager, Phys. Rev.65, 117 (1944).

[4] R. M. White, Quantum Theory of Magnetism, McGraw-Hill, New York 1970.

[5] A. Auerbach, Interacting Electrons and Quantum Mag- netism, Springer-Verlag, New York 1994.

[6] F. Igl´oi, J. Phys. A: Math. Gen.20, 5319 (1987).

[7] C. Vanderzande and F. Igl´oi, J. Phys. A: Math. Gen.20, 4539 (1987).

[8] F. C. Alcaraz and M. N. Barber, J. Stat. Phys.46, 435 (1987).

[9] Th. Wittlich, J. Phys. A23, 3825 (1990).

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Quant. Inf.1, 189 (2003).

[11] J. K. Pachos and M. Plenio, Phys. Rev. Lett.93, 056402 (2004).

[12] H. E. Brandt, Nonlin. Anal. Theo. Meth. Appl.71, e474 (2009).

[13] H. Jiang and X.-M. Kong, ‘Thermodynamics Prop- erties and Phase Diagrams of Spin-1 Quantum Ising Systems with three-Spin Interactions’, (2011) doi:arXiv:1111.4888v1.

[14] H.-L. Wang, Y.-W. Dai, B.-Q. Hu, and H.-Q.

Zhou, ‘Bifurcation in ground-State Fidelity for a one-Dimensional Spin Model with Compet- ing two-Spin and three-Spin Interactions’, (2011) doi:arXiv:1106.2114v1.

[15] B. P. Lanyon, C. Hempel, D. Nigg et al., Science334, 57 (2011).

[16] M. Topilko, T. Krokhmalskii, O. Derzhko, and V. Ohan- yan, Eur. Phys. J. B85, 278 (2012).

[17] X. Zhang, A. Zhang, and F. Li, ‘Detecting multi-Spin Interaction of an XY Spin Chain by Geometric Phase of a Coupled Qubit’, (2012)doi:arXiv:1204.2627v1.

[18] P. K. Aravind, Found. Phys. Lett.15, 397 (2002).

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[20] W.-H. Steeb and Y. Hardy, Matrix Calculus and Kro- necker Product: A Practical Approach to Linear and Multilinear Algebra, second edition, World Scientific, Singapore 2011.

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[22] M. A. Nielsen and I. L. Chuang, Quantum Comput- ing and Quantum Information, Cambridge University Press, Cambridge 2000.

[23] Y. Hardy and W.-H. Steeb, Classical and Quantum Computing with C++ and Java Simulations, Birkhauser Verlag, Basel 2002.

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[25] N. D. Mermin, Quantum Computer Science, Cam- bridge University Press, Cambridge 2007.

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[26] Peres A., ‘Quantum Entanglement: Criteria and Collec- tive Tests’,http://xxx.lanl.gov/quant-ph/9707026.

[27] A. Wong and N. Christensen, Phys. Rev. A63, 044301 (2001).

[28] W.-H. Steeb and Y. Hardy, Quantum Mechanics using Computer Algebra, second edition, World Scientific, Singapore 2010.

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