Asian monsoon - an important pathway into the stratosphere ?
Paul Konopka
Forschungszentrum J ¨ulich, Germany,
Institute for Energy and Climate Research - Stratosphere (IEK-7) P.Konopka@fz-juelich.de
Outline
Motivation - why should we care about the Asian Summer Monsoon (ASM)
Modeling of transport and chemistry with CLaMS:
Lagrangian view transport
numerical diffusion versus physical mixing entropy (potential temperature) as vertical coordinate
CLaMS: some applications
ASM as a pathway of transport into the Tropical Tropopause Layer (TTL)
Conclusions
Monsoon in the tropical troposphere
...is defined as seasonal reversing wind accompanied by corresponding changes in precipitation associated with asymmetric heating of land and sea (Wikipedia)
Tropospheric cyclone drives the anticyclone above
Summer convection + Coriolis force + Kelvin’s circulation theorem ⇒
Convergent flow in the troposphere ⇒ cyclone Divergent flow in the UTLS ⇒ anticyclone
courtesy of Yong Wang
Randel and Park, JGR, 2006:
GPH and MPV at 150 hPa AIRS H2O and O3 at 360 K
Asian summer monsoon anticyclone
≈nearly stationary disturbance of the
...this high pressure system in the upper troposphere extends well into the lower stratosphere up to about 20 km (orθ =420 K)
Randel and Park, JGR, 2006
Park et al., JGR, 2007:
strongly isolated anticyclone between 12 and 20 km, (from ACE-FTP data)
Haynes and Shuckburgh, JGR, 2000:
weak and permeble NH STJ during summer (from the effective diffusivity concept)
Dethof at al., QJRMS, 1999:
Bannister at al., QJRMS, 2004:
Gettelman et al., JGR, 2004:
Levine et al., JGR, 2007:
James et al., GRL, 2008:
strong contribution to the moist phase of the tape-recorder
2-month (July and August) aver- age NCEP zonal wind (shaded) and temperature anomalies (thin lines, deviation from zon. mean)
Asian summer monsoon: Why we should care ?
Park et al., JGR, 2007
Asian summer monsoon: Why we should care ?
HCN at 13.5 km, JJA Randel et al., Science, 2010 ...the monsoon circulation provides an effective pathway for pollution from Asia, India, and Indonesia to enter the global stratosphere...
...mainly SO2, but also H2O
averaged between 0 and 100 E
Asian summer monsoon: Why should we care ?
...the most populated and po- luted area on Earth, more than half the world’s population
...the strongest influence of the Earth orography on the compo- sition of the atmosphere
courtesy of Yong Wang dominated by orographic insula-
tion of the Himalaya (Boos and Kuang, Nature, 2010)
Objectives
Impact of the Asian summer monsoon on the distribution of CO, HCN, SO2, H2O, O3, and aerosols in the Tropical Tropopause Layer (TTL), i.e. at the “gateway” into the stratosphere
In particular:
How important is the isentropic transport from the extratropics (from the northern summer hemisphere) into the TTL (in-mixing) ?
(e.g. Chen et al., 1995, Dunkerton et al., 1995, Hayens and Shuckburgh, 2005, JGR)
Winter
TTL
Upwelling
380 K 350 K 420 K
Summer
In−mixing
Tropopause
Modeling with CLaMS
CLaMS - Lagrangian Chemistry Transport Model with ≈ 106 air parcels
air parcel = “pivotal point with mixing ratios µi, of m species with i = 1, ..., m”
Potential temperature/pressure as vertical coordinate in the stratosphere/troposphere Horizontal meteor. winds (ECMWF, NCEP, WACCM)
Vertical velocity: diabatic approach (θ˙ from radiation, latent heat rather than p)˙ Lagrangian mixing
Full stratospheric and
simplified tropospheric chemistry
Lagrangian particle sedimentation scheme parallelized code (JUMP)
McKenna et al., JGR, 2002, Konopka et al., JGR, 2004, Grooß et al., 2005, ACP, Konopka et al., 2007, 2010, ACP
Mixing Trajectory
Chemistry
Sedimentation
0000 00 1111 11 0000
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Euler versus Lagrange
Left: Casper David Friedrich: Wan- derer above the Sea of Fog
Bottom: Montgolfier ballon over Ro- camadour
Lagrangian view of transport
Mixing Chemistry
Advection
Chemistry Advection
driven by given wind fields
along the trajectories
Tracer
transport =
Advection
(Trajectories) (reversible)
+
Mixing
(Adaptive grid)
(irreversible)
Euler versus Lagrange
To solve: ∂tni + ∇ · (niu) = 0, niu = niu¯ + niu′, niu′ = D∇ni (Fick’s law)
ni - number densities of species i, i=0,...,m, u¯ - velocity of the flow, D - diffusion coefficient,
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
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00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 0
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 1
000000000000000000000000000 111111111111111111111111111
000000000000000000000000000 111111111111111111111111111
000000000000000000000000000 111111111111111111111111111
000000 000000 000000 000000
111111 111111 111111 111111
00000 00000 00000 00000 00000 00000 00000 00000
11111 11111 11111 11111 11111 11111 11111 11111
00000 00000 00000 00000 00000 11111 11111 11111 11111 11111
0000000 0000000 0000000 0000000 1111111 1111111 1111111 1111111
0000 0000 0000 0000 0000 00
1111 1111 1111 1111 1111 11
000000 000000 000000 000000 000000 000
111111 111111 111111 111111 111111 111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
000000 000000 000000 000000 000000 000000 000000 000000
111111 111111 111111 111111 111111 111111 111111 111111
0000 0000 0000 0000
1111 1111 1111 1111
000000 000000 000000 000000 000
111111 111111 111111 111111 111
00000000 00000000 00000000 0000
11111111 11111111 11111111 1111
00000 00000 00000 00000 11111 11111 11111 11111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
00000000 00000000 00000000 11111111 11111111 11111111
0000000 0000000 0000000 1111111 1111111 1111111
00 11
00 11
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11 00 11
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0000 0000 0000
1111 1111 1111 1111
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0000 0000 0000 0000 0000
1111 1111 1111 1111 1111
00000000 00000000 0000 11111111 11111111 1111000000000000000000
111111 111111
111111 00000000000000000000000000000000000000000000000000000000 11111111 11111111 11111111 11111111 11111111 11111111 11111111
000000 000000 000000 000000
111111 111111 111111 111111
00000000 00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 11111111 1111
000000 000000 000000 111111 111111 111111
Euler versus Lagrange
To solve: ∂tni + ∇ · (niu) = 0, niu = niu¯ + niu′, niu′ = D∇ni (Fick’s law)
ni - number densities of species i, i=0,...,m, u¯ - velocity of the flow, D - diffusion coefficient, Eulerian reference frame is a way of looking at
fluid motion that focuses on specific points in the space through which the fluid moves
(regular grid)
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
000000 000000 000000 000000 000000 111111 111111 111111 111111 111111
000000 000000 000000 000000 111111 111111 111111 111111
0000 0000 0000 0000 0000 00
1111 1111 1111 1111 1111 11
00000000 00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000 00000 00000 00000 00000 00000 00000 00000
11111 11111 11111 11111 11111 11111 11111 11111
0000 0000 0000 0000 00
1111 1111 1111 1111 11
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 0000
11111111 11111111 11111111 1111
00000 00000 00000 00000 11111 11111 11111 11111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
00000 00000 00000 00000 00000 00000 00000 00000
11111 11111 11111 11111 11111 11111 11111 11111
00000000 00000000 00000000 11111111 11111111 11111111
000000 000000 000000 111111 111111 111111
Physical mixing D “overloaded” by numerical diffusion ∼ ∆x2/∆t ≈ 106m2/s ≫ D, for
∆x = 100 km, ∆t = 10 min (Courant criterion)
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0000 0000 0000
1111 1111 1111 1111
0000 1111
0000 0000 0000 0000 0000
1111 1111 1111 1111 1111
00000000 00000000 0000 11111111 11111111 1111000000000000000000
111111 111111
111111 00000000000000000000000000000000000000000000000000000000 11111111 11111111 11111111 11111111 11111111 11111111 11111111
000000 000000 000000 000000
111111 111111 111111 111111
00000000 00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 11111111 1111
000000 000000 000000 111111 111111 111111
Euler versus Lagrange
To solve: ∂tni + ∇ · (niu) = 0, niu = niu¯ + niu′, niu′ = D∇ni (Fick’s law)
ni - number densities of species i, i=0,...,m, u¯ - velocity of the flow, D - diffusion coefficient, Eulerian reference frame is a way of looking at
fluid motion that focuses on specific points in the space through which the fluid moves
(regular grid)
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11
00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00 00
11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 11 0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
0000000000000000000000000000 1111111111111111111111111111
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
000000 000000 000000 000000 000000 111111 111111 111111 111111 111111
000000 000000 000000 000000 111111 111111 111111 111111
0000 0000 0000 0000 0000 00
1111 1111 1111 1111 1111 11
00000000 00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000 00000 00000 00000 00000 00000 00000 00000
11111 11111 11111 11111 11111 11111 11111 11111
0000 0000 0000 0000 00
1111 1111 1111 1111 11
00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 1111
00000000 00000000 00000000 0000
11111111 11111111 11111111 1111
00000 00000 00000 00000 11111 11111 11111 11111
00000000 00000000 00000000 00000000
11111111 11111111 11111111 11111111
00000 00000 00000 00000 00000 00000 00000 00000
11111 11111 11111 11111 11111 11111 11111 11111
00000000 00000000 00000000 11111111 11111111 11111111
000000 000000 000000 111111 111111 111111
Physical mixing D “overloaded” by numerical diffusion ∼ ∆x2/∆t ≈ 106m2/s ≫ D, for
∆x = 100 km, ∆t = 10 min (Courant criterion)
Lagrangian reference frame is a way of look- ing at fluid motion where the observer follows individual fluid particles as they move through space and time
(irregular grid)
00 11
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11 00 11
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000000 000000 000000 000
111111 111111 111111 111111 111
0000 1111
000000 000000 000000 000000 000000
111111 111111 111111 111111 111111
00000 00000 00000 00000 00000 11111 11111 11111 11111 11111000000000000000000000
111111 111111 111111 111
0000000 0000000 0000000 0000000 0000000 0000000 0000000
1111111 1111111 1111111 1111111 1111111 1111111 1111111
0000 0000 0000 0000 00
1111 1111 1111 1111 11
000000 111111
00000000 00000000 00000000 00000000 00000000 0000
11111111 11111111 11111111 11111111 11111111 1111
00000 00000 00000 11111 11111 11111
r(t)
Mixing is under control. Advection means cal- culation of trajectories
dr(t)
...numerical diffusion versus
atmospheric mixing
Stratospheric stirring
...stratospheric transport is dom- inated by horizontal winds. Due to a strong stable stratification, the vertical motion is supressed.
...stratosphere looks like mixing colors with a stir- ring stick.
Euler versus Lagrange
t=t
t=t
t=t
t=t
1
2
3
4
u
Eulerian grid
...one of the most intriguing features offered by the La- grangian transport is the possibility to to parameterize the “true” physical mixing in terms of the numerical dif- fusion...
Grid adaptation ⇒ mixing
A C B
quasiuniform distribution of air parcels
Delaunay triangulation ⇒ next neighbors
Grid adaptation ⇒ mixing
A C B
quasiuniform distribution of air parcels
Delaunay triangulation ⇒ next neighbors
sheared flow
∆t = 6 − 24 hours
Grid adaptation ⇒ mixing
A C B
quasiuniform distribution of air parcels
Delaunay triangulation ⇒ next neighbors
sheared flow
∆t = 6− 24 hours
A C B
D
grid adaptation =
regridding of the deformed grid
⇒ new air parcels
⇒ interpolations (num. diffusion)
⇒ mixing
So, how to proceed ?
Two problems have to be solved:
To find an appropriate (irregular) Lagrangian grid (i.e. parameters ∆r and ∆z). The numerical diffusion due to the interpolations within such a grid can be estimated as
Dnumh ≈ ∆r2/∆t Dvnum ≈ ∆z2/∆t.
and, consequently:
Dhnum
Dvnum = ∆r2
∆z2 = α2 = Dh
Dv
, α = ∆r
∆z aspect ratio
Dv, Dh - ‘true” vertical and horizontal diffusivities in a horizontal and stably stratified flow (Haynes and Anglade, JGR, 1997).
So, how to proceed ?
...and the second problem is:
To find a (physical) mechanism how to trigger such interpolations. Here, we follow the idea of the gradient Richardson number:
Ri = N2
∂u
∂z
2
+
∂v
∂z
2 i.e. mixing occurs only for sufficiently small values of Ri < Ric
with u, v denoting the horizontal wind components and N the Brunt Vaisala frequency.
...i.e. mixing happens either when the wind shear is great enough to overpower any stabilizing buoyant forces (denominator is large), or when the dry or, more general, moist environment is static instabile (numerator is small or even negative).
1st step:
to choose the right grid...
(Konopka et al., Geophysical Monograph Series, 2012)
Entropy and static stability based grid
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1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111 1111111111111111111
320 K 350 K
360 K
450 K
380 K 420 K
600 K
Tropopause
UTLS
TR ST
High Latitudes
TR UTLS ST
TR UTLS ST
Mid−Latitudes Tropics
Stratosphere (Overworld)
ST
TR
UTLS
S
S = = S
Vα > V < < V
α > α
<
<
“Same entropy per air parcel”
Sap = ∆r2∆z s(θ, ρ) = const, s(θ, ρ) = cpρln θ θ0
“Aspect ratio proportional to static stability”
α = ∆r
∆z ∼ N, N2 = g θ
dθ
dz (Brunt Vaisala frequency)
Why entropy ?
0000000000000000 0000000000000000 0000000000000000 0000000000000000 0000000000000000 0000000000000000 0000000000000000 0000000000000000 0000000000000000
1111111111111111 1111111111111111 1111111111111111 1111111111111111 1111111111111111 1111111111111111 1111111111111111 1111111111111111 1111111111111111
Stratosphere
Troposphere Mesosphere
S T
T
∆
ref
ref S + Sref
adiabatic
∆ S
∆ S
∆ S
Carnot cycle
"same available work"
...in a system where no additional information is available, same entropy means that each air parcel contains the same amount of available energy that is transferable into work that manifests as atmospheric motion. Such motion may irreversibly dissipate into friction.
Definition of the grid
Thus:
nap = 1
∆r2∆z = s Sap
α = ∆r
∆z = kN nap - density of air parcels
α - aspect ratio
∆r =
kN Sap
s
13
∆z =
1
kN
23
Sap
s
13
N and s examplary de- rived from ERA-Interim for 1.01.2002.
Scaling properties
Vertical diffusivity Dv per mixing event ⇒
Vertical diffusivity Dv per volume unit ⇒
N and s examplary de- rived from ERA-Interim for 1.01.2002.
2st step:
to trigger mixing by
physical parameters...
Lyapunov exponent λ
r0
t=t0
Consider an air parcel sur- rounded by a small circle of ra- dius r0.
t=t + t r r
+
−
0
After a time ∆t and for sufficiently small values of r0, the circle is deformed into an ellipse with minor and major axes r− and r+
Lyapunov exponent λ
r0
t=t0
Consider an air parcel sur- rounded by a small circle of ra- dius r0.
t=t + t r r
+
−
0
After a time ∆t and for sufficiently small values of r0, the circle is deformed into an ellipse with minor and major axes r− and r+
Definition: (Lyapunov exponent)
λ± = ± 1
∆t ln r± r0
for sufficiently small ∆t and r0
Incompressible flows ⇒ (r02 = r−r+) ⇒ λ− = λ+
Dynamically adaptive grid
Before the advection step
A C B
Determine nearest neighbors (e.g. for point A), r0 - mean distance between air parcels
Set the critical Lyapunov exponent λc
and the time step ∆t (free parameter) Define rc±
r±c = r0 exp±λc∆t
Dynamically adaptive grid
Before the advection step
A C B
Determine nearest neighbors (e.g. for point A), r0 - mean distance between air parcels
Set the critical Lyapunov exponent λc
and the time step ∆t (free parameter) Define rc±
r±c = r0 exp±λc∆t
After the advection step
A C B
D
If r > r+c , then a new grid point D is inserted midway between A and B (insertion)
If r < rc−, then grid points A and C are removed and a new grid point is intro- duced midway between the positions of A and C (merging)
Mixing in CLaMS
Large-scale wind
Small-scale deformations
Filamentation
Mixing
(irreversibility)
Mixing in the vicinity of the subtropical jet
Subtropical jet
over Himalayas
Mixing in the vicinity of the subtropical jet
Subtropical jet over Himalayas
Strong
deformations ...
Mixing in the vicinity of the subtropical jet
Subtropical jet over Himalayas
... and mixing !
Pan et al., 2006, JGR
λ c - “critical Lagran-
-gian deformation”
A completely different view...
...regular (Euler)
A completely different view...
...regular (Euler)
versus irregular (Lagrange)
courtesy of Rolf Müller
...and chemistry
species lower boundary upper boundary
CH4 CMDL HALOE
Mean Age linear source MIPAS (SF6)
CO2 CMDL Mean Age
CO CMDL + MOPITT Mainz-2D
O3 0 HALOE, θ ≥ 500 K
O3 (tracer) 0 HALOE, θ ≥ 500 K
HCl 0 HALOE, θ ≥ 500 K
H2O ECMWF, θ ≤ 280 K HALOE
N2O, F11 CMDL (CATS) 0
HCN MODIS 0
Simplified chemistry
CH4 ⇒ (OH, O(1D), Cl) ⇒ H2O, CO ⇒ (OH) ⇒ CO2
(hν) ⇒ O3 ⇒ (HOx) ⇒, N2O, F11 ⇒ (O(1D), hν) ⇒ HCN ⇒ (OH, O(3D), uptake by the ocean)⇒
Multi-annual CLaMS simulations (2001-10)
- HALOE - Climatology:
Grooss and Russell, ACP, 2005 - CMDL: GLOBALVIEW, 2007 CO2/CH4/CO since 1979/84/91 P. Tans, K. Masarie, P. Novelli - CMDL: CATS (4 stations) N2O, F11, J. Elkins
- MIPAS, SF6-Age Stiller et al., ACP, 2008 - MOPITT (V3, V4)
Pommrich at al., PhD, 2008 - HCN
Pommrich at al., GRL, 2010
...isentropic thinking
diabatic rather than kinematic vert. velocities
potential temperature θ defines the vertical coordinate
Cross isentropic velocity θ˙ derived from diabatic processes (long- and shortwave radiation with clouds + laten heat +,...),
⇒ σ-θ, hybride ζ-coordinate (Mahowald et al., JGR, 2002)
diabatic rather than kinematic vert. velocities
potential temperature θ defines the vertical coordinate
Cross isentropic velocity θ˙ derived from diabatic processes (long- and shortwave radiation with clouds + laten heat +,...),
⇒ σ-θ, hybride ζ-coordinate (Mahowald et al., JGR, 2002)
p [hPa]
340 360 380
310
280 100
200
300
500
1013
[K]
0.12
0.25
0.80 0.40
1.00
θ =p/p
s10 30 50 70
[deg N]
Subtropical Jet σ
ζ = θ (pot. Temp.) above 300 hPa
dζ
dt = dθdt
diabatic rather than kinematic vert. velocities
potential temperature θ defines the vertical coordinate
Cross isentropic velocity θ˙ derived from diabatic processes (long- and shortwave radiation with clouds + laten heat +,...),
⇒ σ-θ, hybride ζ-coordinate (Mahowald et al., JGR, 2002)
p [hPa]
340 360 380
310
280 100
200
300
500
1013
[K]
0.12
0.25
0.80 0.40
1.00
θ =p/p
s10 30 50 70
[deg N]
Subtropical Jet σ
ζ = θ (pot. Temp.) above 300 hPa
dζ
dt = dθdt
ζ ∼ σ = p/ps, p - surf. pressure below 300 hPa
dζ = ˙σ