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ISOARC project: From source to sink - Monitoring the isotopic fingerprints of Arctic moisture

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Introduction

In recent years, a new generation of analyzers (CRDS) has been used to develop an observing network of the isotopic composition of atmospheric water vapour (δ18O, δD, leading to d-excess = δD - 8.δ18O) in the Arctic, aiming at documenting the isotopic fingerprint of the hydrological cycle [Bonne et al.

2015, Steen-Larsen et al. 2013, 2015]. The interest of observations at the moisture sources also lead to regular ship based measurements in the Atlantic realm [Benetti et al. 2017].

To identify the eastern Arctic moisture sources, two analyzers are continuously operating since July 2015 on-board Polarstern research vessel (close to the

evaporation sources) and in the ground station of

Samoylov (Lena delta, 72°22’N, 126°29’E).

Jean-Louis Bonne1, M. Werner1, Hanno Meyer1, S. Kipfstuhl1, B. Rabe1, M. Behrens1, L. Schönicke1, H. C. Steen-Larsen2 / 1AWI Germany, 2CIC Denmark

ISOARC project: From source to sink - Monitoring the isotopic fingerprints of Arctic moisture

BREMERHAVEN

Am Handelshafen 12 27570 Bremerhaven Telefon 0471 4831-0 www.awi.de

References

- Benetti et al. Stable isotopes in the atmospheric marine boundary layer water vapour over the Atlantic Ocean, 2012–2015. Sci. Data 4:160128 doi: 10.1038/sdata.2016.128 (2017).

- Bonne et al. 2015: The summer 2012 Greenland heat wave: in situ and remote sensing observations of water vapour isotopic composition during an atmospheric river event, J. Geophys. Res.

Atmos., 120, doi:10.1002/2014JD022602.

- Steen-Larsen et al. 2013: Continuous monitoring of summer surface water vapor isotopic composition above the Greenland Ice Sheet, Atmos. Chem. Phys., 13, 4815-4828.

- Steen-Larsen et al., 2015: Moisture sources and synoptic to seasonal variability of North Atlantic water vapor isotopic composition, J. Geophys. Res. Atmos.,120, 5757–5774, doi:10.1002/2015JD023234

Acknowledgements - AWI strategic fund

- Polarstern expediton PS93-1 (Grant No. AWI-PS93.1_02) - R. Krocker, P. Gerchow, E. Dunker and colleagues

- A. Astapov, S. Tippenhauer, M. Hoppmann, H. Hampe, R. Engelmann, S. Bohlmann, S. Arndt, L. Rossmann, L. Lembke-Jene, V.

Schlindwein, M. Horn, M. Haarig, H. Kalesse, E. Burkhardt, M. Flau, B. Christian, J. Goedecke.

Contact: jean-louis.bonne(at)awi.de, orcid.org/0000-0001-7090-2147

Summary and perspectives

Our studies have demonstrated the ability to measure vapour isotopic composition in a wide range of humidity values, from polar to tropical regions. Humidity is following temperatures to the first order.

The most depleted isotopic values are observed over sea ice from Polarstern and in Arctic winter in Samoylov. Isotopic values are more depleted in Samoylov than above the open ocean, showing the impact of atmospheric transport.

ECHAM5-wiso model correctly simulates humidity and temperature from both observational datasets. The vapour isotopic composition is well reproduced above the open ocean at every latitude, but needs to be improved at sea ice (Fig. 3).

At Samoylov station (Fig. 4), which is also influenced by continental air masses and local moisture sources, generally higher biases are seen, especially in spring. These maybe linked to snow melt and continental recycling (ice break-up).

Different Arctic records (Fig.1) could be combined to track vapour along atmospheric transport patterns [as in Bonne et al.

2015]. The measurements performed in a station in the Arctic region will help differentiating between long-distance vapour transport and local moisture contributions.

Arctic Atlantic Antarctica Atlantic Arctic

North Pole

East Greenland coast

Arctic sea ice Arctic sea ice Antarctic sea ice

ITCZ ITCZ

Bremerhaven Cape Town Punta Arenas Bremerhaven Bremerhaven

Polarstern

Fig.5: Samoylov 6-hours averaged observations (blue) & ECHAM5-wiso model outputs (red) from 07-2015 to 11-2016. Downwards: temperature, specific humidity, δ18O, d-excess, sea ice cover (at 500 km from Samoylov).

Fig.4: Simulated moisture transport over the Arctic Ocean towards Samoylov on 2015-09-30: amount of transported moisture (left) and evaporation minus precipitation (right), estimated from modelled 10-days Flexpart Lagrangian backtrajectories.

Fig.2 (left): Map of Polarstern positions at 6 hours interval from 07-2015 to 11-2016.

Iceland

Bergen

Ny Ålesund

Labytnangy Igarka

Samoylov

Polarstern

δ18OδD

Samoylov

Samoylov

Fig.3: Polarstern observations (blue) and colocated ECHAM5-wiso model outputs (red) from 07-2015 to 11-2016 at 6 hours resolution. Downwards:

temperature, specific humidity, δ18O, d-excess, latitude, local sea ice cover.

Fig.1 (right): Concept of the ISOARC project, with the current Arctic network of vapour isotopic analyzers.

Samoylov

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