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Nanomagnetism,oxides and resonance laboratory

Service de Physique de l’Etat

Condensé

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9 permanent researchers

4 technicians, 2 electronic engineer

5 PhD students , 5 post-docs

+Associated teams for Neutrons and NMR

The team

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• Magnetism at small scales

– Thin films and nanostructures – Transport

– Dynamics

• Oxides (superconductors and multiferroics)

• Mössbauer, NMR and NQR

• Spin electronics based magnetic sensors

Research axis

0 100 200 300 400

0 100 200 300

ρ (μΩ.cm)

T (K)

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Synthesis and characterization

of cuprates, iron-pnictides and multiferroic oxides

A. Forget, D. Colson

Single crystal growth by flux

Synthesis of ceramics by solid state reaction

BiFeO3 :1 ferroelectric domain crystal

A multiferroic with Ps= 100 μC/cm2 at 300K !

0 100 200 300 400

0 100 200 300

ρ (μΩ.cm)

T (K)

First single crystals of mercury cuprates (1994)

Tc=95K for HgBa2 CuO4+d

PS[111]

K+: 4s1

Hole doped (Tcmax ~ 38K)

Ru2+:4d75s1 Isolelectronic of Fe

Co2+: 3d Ni2+: 3d8 electron‐doped

P3‐: 3s23p3

Isolelectronic of As

(Tcmax ~ 25K)

Iron pnictide superconductor Ba(Fe1-x Mx )2 As2 single crystals

Characterization:

X-ray mesasurements, thermogravimetric analysis Squid magnetometry

Lebeugle D., Colson D., Forget A., Viret M, Appl.

Physics Lett. 91 22907 (2007)

Raman: Gallais, Y.; Le Tacon, M.; Sacuto, A.; Colson, D, Europhysics Letters (2006), 73(4), 594-600.

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Transport Properties in Superconducting High-T

c

Cuprates and Iron-based Pnictides

Measurements of resistivity, Hall effect and magnetoresistance

Study of the transport properties in Co and Ru substituted Ba2 Fe2 As2

-1.5 -1 -0.5 0 0.5 1

RH (10-9 m3 /C)

0 0.05 0.19 0.44

0.26

0.35 Ba(Fe

1-xRu

x)

2As

2

(a)

-3 -2.5 -2 -1.5 -1 -0.5

0 50 100 150 200 250 300

RH (10-9 m3/C)

T (K) 0.014 0 0.06

0.07 0.12 0.2

Ba(Fe

1-xCo

x)

2As

2

(b)

Evidence for different contributions of electrons and holes to the transport properties

Determination of superconducting fluctuations in YBa2 Cu3 O6+x by high-field magnetoresistance measurements

In the optimally doped sample, the pseudogap temperature is below the onset of superconducting fluctuations (SCF)

The pseudogap phase cannot be considered as a percursor state for superconductivity

Hole doping nh T

?

Pseudogap line

SCF SC F. Rullier-Albenque, D. Colson, A. Forget, H. Alloul, PRL 103,057001 (2009)

F. Rullier-Albenque, D. Colson, A. Forget et al., PRB 81, 224503 (2010).

F. Rullier-Albenque, H. Alloul, G. Rikken, PRB 84, 014522 (2011).

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Photovoltaic effect of BiFeO3 single crystals

0 5 0 10 0 150 2 00 25 0

-0,3 -0,2 -0,1 0,0 0,1 0,2

BFO BFOBFO

BFO BFO

E1

I (nA)

T im e (m in )

E1

E2 E2

E1

E2 E1

E2

E1

B iFeO3

s in g le cry s tal G o l d e le c tr o de

V A

Sp a c i ng o f 2 5 µ m

G l a ss pl a te

Multiferroics

Photostriction inBiFeO3

BiFeO3 is ferroelectric and antiferromagnetic Photons related effects

B. Kundys, M. Viret, D. Colson and D. O. Kundys, Nature Materials 9, 803 (2010).

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Magnetic atomic contacts

0 3 6 9 12 15

-1 -0.8 -0.6 -0.4 -0.2 0

d (nm) σ (2e2 /h)

Ferromagnetic resonance

In atomic contacts and nanobridges

A. Ben Hamida, O Rousseau, S Petit-Watelot and M Viret, Europhys. Lett. 94, 27002 (2011).

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Dynamics of a magnetic Vortex probed by MRFM

Low temperature MRFM:

- magnetic nanoparticles - new materials

Magnetization dynamics in spin transfer nano-oscillators

Experimental development

Vortex core reversal induced by RF pulses

Identification of the spin-wave modes

Magnetization dynamics in nannostructures

B. Pigeau, et al, Nature Physics, 7, 26-31 (2011).

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-0.008 -0.006 -0.004 -0.002 0 0.002 0.004 0.006 0.008

0 50 100 150 200 250 300 350 400

2D Compas for watch Magnetic imaging,NDE Current sensors for fuel cells

Read heads, current sensors for electricity meters and failure surveillance, Rotational switches

Spin electronics based Magnetic sensors

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Biochips

Sensors for medical applications

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Femto Tesla sensors for low field MRI and biomagnetism

Sensors for medical applications

Common MEG lab at Neurospin

Magneto Cardiography Very low field MRI

Referenzen

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