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Entanglement properties

5.1 Tripartite entanglement

Despite the great importance of entanglement, a necessary and sufficient condition for the entanglement of a given state is only known for two-qubit systems [46]. The determina-tion of entanglement for multipartite states, however, is an open quesdetermina-tion. For three qubits it was shown in Ref. [47] that two different kinds of genuine multipartite entanglement (i.e. each party is entangled with each other party) can occur. Namely, each tripartite entangled state can (with nonzero probability) be converted2 by LOCC [48] to either one of two standard forms, the GHZ state, |GHZi = 1

2(|↑↑↑i+|↓↓↓i) [49], or the W state,

|Wi = 1

3(|↑↑↓i+|↑↓↑i+|↓↑↑i), which are mutually unrelated under LOCC. For GHZ-like entanglement, a measure was invented [50], the3-tangle τ. It allows for a reliable distinction between the two classes of entanglement, as it is zero for all W-type states (and all separable states, of course), whereas it is greater than zero for all states in the GHZ class. An expression forτ in terms of the coefficients of the state in the standard basis is given in appendix D.1.

A tool for detection of any kind of genuine tripartite entanglement for arbitrary states is not at hand; however, if some knowledge about the state under investigation is provided, entanglement witnesses (EW) can be used [51, 52]. These are observables with a positive ex-pectation value for all (bi-)separable states (in generaln−1 partite entangled states), whereas a negative expectation value indicates the presence of tripartite (n-partite) entanglement3. The common way to construct an EW for a state|ψi is

W =α1l− |ψihψ|, (5.1)

whereα is the maximal squared overlap of |ψiwith any biseparable or fully separable state.

Determination of α is in general complicated4, but we can use the proximity of the states under investigation (as described in 3.3.2 and 3.4) to W and GHZ states, respectively, to make use of known values forα. In order to measure EWs, they must be decomposed into a sum of local measurements. This as well is a demanding task and we will again refer to previous work done on this topic [55, 56, 57].

5.1.1 Entanglement of state |E3i

As pointed out in 3.4.1,|E3i is for zero energy bias close to|GHZi= 1

2(|↑↑↑i+|↓↓↓i). For constructing a GHZ witness adapted to|E3i, the maximal squared overlap of|E3i with non-GHZ entangled states is required, though not known. We therefore choose an EW suitable for detecting the state|GHZifor whichαis known (α= 3/4) and thus make use of the proximity of|E3i to|GHZi. However, instead of using the EW [58]

WfGHZ = 3

41l− |GHZihGHZ|, (5.2)

2No operational criterion for the existence of such a transformation between two given states is known.

3The object of study here is tripartite entanglement. However, the concept of entanglement witnesses applies to multipartite entanglement as well.

4Since one has to minimize over all product states, i.e. over a convex hull of states, numerical calculations involving the theory of convex optimization are commonly used [52, 53, 54].

5.1Tripartite entanglement 41

Figure 5.1: 3-tangle and expectation value of the GHZ witness WGHZ (explicit form in the text) for the state |E3i. As can be seen, both quantities indicate a strong GHZ-like entanglement around²= 0.

-1 -0.75 -0.5 -0.25 0 0.25 0.5 0.75 1

Figure 5.2: 3-tangle and expectation value of the Bell operator ˆMGHZ (explicit form in the text) for the state |E3i. The high 3-tangle coincides with a significant violation of the Bell inequality.

we apply an EW introduced in Ref. [57], which can be measured with two collective local measurement settings,

The two local settings here are the© ˆ these, all correlators appearing in (5.3) can be computed. In contrast, the EWWfGHZ requires four measurement settings (see table 5.1).

The 3-tangle τ(|E3i) and the expectation value hE3|WGHZ|E3i for varying energy bias are shown in figure 5.1. Both quantities indicate a strong (cp. limiting case: τmax=τ(|GHZi) = 1,hWGHZimin =hGHZ|WGHZ|GHZi=−3/4) tripartite entanglement of GHZ type in a narrow range around zero energy bias (here, only|E3iis plotted,|E4ishows the same behavior). The range of negative expectation value forWGHZis even a little smaller than the range of non-zero 3-tangle. This reflects the fact that EWs need to be adapted to the state under investigation and can take positive expectation value even if the associated entanglement is present. In section 5.2, we will comment on the violation of Bell inequality as displayed in figure 5.2.

5.1.2 Entanglement of state |E2i

More GHZ-like states can be found among the eigenstates. In figure 5.3, the 3-tangleτ(|E2i) and the expectation values for two EWshE2|W(1)

GHZ|E2iandhE2|W(2)

GHZ|E2ifor varying energy bias are displayed. We obtain a strong (limiting case: hW(1)

GHZimin = hW(2)

GHZimin = −1/4) entanglement for a finite energy bias ² ≈ ±2.6∆ and a high residual entanglement in the range between these two maxima.

42 5 Entanglement properties

Figure 5.3: 3-tangle and expectation value of the GHZ witnessesWGHZ(1) and WGHZ(2) for the state|E2i. For finite energy bias ²≈ ±2.6∆, we find a peaking 3-tangle as well as nega-tive expectation value for the two GHZ wit-nesses, indicating entanglement of the GHZ class. Moreover, the entanglement is more robust to detuning of the energy bias com-pared to the situation for|E3i.

-8 -6 -4 -2 0 2 4 6 8

Figure 5.4: 3-tangle and expectation value of the Bell operator ˆMGHZfor the state|E2i.

A significant violation of the corresponding Bell inequality over a relatively large range of ²can be observed.

Left maximum at ²≈ −2.6∆

The explicit form of the state constituting the left maximum is

|E(1)2 i=−α©

Thus, this state is close to the state

|GHZi= 1

onto the state|GHZi has the form UˆE(1)2 =eiπ/4

nRˆx(−π/2) ˆRz(−π) ˆRy(π/2) o⊗3

. (5.7)

The EW is chosen such as to detect tripartite entanglement in the proximity of|GHZi[56], W(1)

GHZ = 3

41l− |GHZihGHZ|= 3

41l−UˆE(1)2 |GHZihGHZ|UˆE(1)2 . (5.8) For an optimal decomposition ofW(1)

GHZ refer to table 5.1.

5.1Tripartite entanglement 43 Right maximum at ²≈2.6∆

For the state in the right maximum we find

|E2(2)i=α©

|↓↓↑i+|↓↑↓i+|↑↓↓i − |↑↑↑iª

−β©

|↑↑↓i+|↑↓↑i+|↓↑↑i − |↓↓↓iª

(5.9) withα andβ as above. |E2(2)i is the totally flipped counterpart to|E2(1)i and therefore shows the same behavior after being flipped back by ˆRx(−π)⊗3,

UˆE(2)2 |E2(2)i ≈ |GHZi with UˆE(2)2 = ˆUE(1)2 Rˆx(−π)⊗3 . (5.10) The corresponding EW looks like

W(2)

GHZ= ˆRx(π)⊗3W(1)

GHZRˆx(−π)⊗3. (5.11)

The optimal decomposition ofWGHZ(2) can again be looked up in table 5.1.

Whereas the behavior of the highest excited states|E3iand |E4ifor vanishing energy bias as described above was expected, we make the surprising observation –referring to figure 5.3–

of the existence of GHZ entangled states also in the parameter regime of finite energy bias.

Moreover, the entanglement shown by|E2i is more stable to deviations from the optimal en-ergy bias than the one of|E3i, overcoming a major drawback caused by the antiferromagnetic nature of the coupling.

5.1.3 Entanglement in the degenerate subspaces

-8 -6 -4 -2 0 2 4 6 8

Figure 5.5: 3-tangle and expectation value of the W witness WW (explicit form in the text) for the state maxL i. The vanishing 3-tangle excludes entanglement of the GHZ type, whereas the negative expectation value of the W witness indicates a W type entan-glement.

Figure 5.6: 3-tangle and expectation value of the Bell operator ˆMW (explicit form in the text) for the state maxL i. The maxi-mal violation of the Bell inequality for the W-equivalent state is not as high as for the GHZ-equivalent states above, however, the violation persists over a large range of ².

In figure 5.5, the 3-tangle and the expectation value of the EWmaxL |WWmaxL ifor the max-imally entangled superpositionLmaxiin the low-energy subspace is displayed (corresponding behavior forHmaxi—not shown separately).

44 5 Entanglement properties

Because we know thatLmaxi(=|E5i) is equivalent under LOCC to the W state (see 3.3.2), we can construct an EW making use of the known maximal overlap (α = 2/3 [58]) between the W state (and therefore the statemaxL i) and biseparable states,

WW = 2

31l− |ψLmaxihψmaxL |. (5.12) Its expectation value is positive on biseparable and fully separable states. It thus detects genuine tripartite entanglement in general, without distinguishing between entanglement of the W and the GHZ class. However, in connection with the 3-tangle, a distinction can be achieved, stating an entanglement of the W type in a large range for².

Reviewing the results of this section, we were able to find states with either kind of genuine tripartite entanglement, GHZ type as well as W type.

EW Local decomposition WfGHZ = 18£

5·1l⊗32 ˆσx⊗3−σˆzσˆz1l−σˆz1l ˆσz1l ˆσzσˆz+12σx+ ˆσy)⊗3+12σxˆσy)⊗3¤ WGHZ = 741l−σˆ⊗3x 12£

ˆ

σzσˆz1l + ˆσz1l ˆσz+ 1l ˆσzσˆz¤ W(1)

GHZ = 161 £

10·1l⊗3+ 4 ˆσ⊗3z 2(ˆσyˆσy1l + ˆσy1l ˆσy+ 1l ˆσyσˆy)σz+ ˆσx)⊗3σz−σˆx)⊗3¤ W(2)

GHZ = 161 £

10·1l⊗34 ˆσ⊗3z 2(ˆσyˆσy1l + ˆσy1l ˆσy+ 1l ˆσyσˆy) + (ˆσz−σˆx)⊗3+ (ˆσz+ ˆσx)⊗3¤ WW = 241 £

17·1l⊗37 ˆσ⊗3x 3(ˆσx1l 1l + 1l ˆσx1l + 1l 1l ˆσx) + 5(ˆσxσˆx1l + ˆσx1l ˆσx+ 1l ˆσxˆσx)−

−(1l−σˆx+ ˆσz)(1l−σˆx23σˆy12σˆz)(1l−σˆx+23σˆy 12σˆz)−

−(1l−σˆx−σˆz)(1l−σˆx+23σˆy+12σˆz)(1l−σˆx23σˆy+ 12σˆz)−

−(1l−σˆx+ ˆσy)(1lˆσx 12σˆy+23σˆz)(1l−σˆx12ˆσy23σˆz)−

−(1l−σˆx−σˆy)(1lˆσx+ 12σˆy23σˆz)(1l−σˆx+12ˆσy+23σˆz)¤ Table 5.1: Local decomposition of the entanglement witnesses used above. The decom-position for WfGHZ (shown to be optimal in [58]) requires four collective measurement settings in contrast to the two settings needed forWGHZ [57]. The optimal decomposi-tion forWGHZ(1) can be found in Ref. [56] (five settings), the one forWGHZ(2) (five settings) was computed by rotating the individual Pauli operators occurring in WGHZ(1) accord-ing to ˆRx(π), WGHZ(2) = ˆRx(π)⊗3WGHZ(1) Rˆx(−π)⊗3. The decomposition for WW (five settings) was obtained similarly from the optimized decompositionWW(1) (five settings) derived in Ref. [55],WW = ˆULWW(1)UˆL.